So, I've been out of Anime for roughly 3 years now and I've been getting that urge to watch it again. Anyone got any good ones that I could start with? Keep in mind, I'm not a big fan of Harem Animes. It's always the same old plot. Though, Shuffle! was an amazing one IMO. I loved that he went for the girl who didn't chase him in the end.
I'm not a fan of Harems myself. I liked Shuffle! a lot too, but really, I don't consider is a harem. When you add Yandere into the mix, I think that nulls it out for me. I'm always down for some Yandere batshit-shit, with the exception being School Days, I hate that so much. Anyway, aside from romances (don't be bashful, it's one of my favorite genres) what are you in to? I'll list some good romance anime, trying to stay away from Harems, but some of like Shuffle, in that you just have to watch them.
Kimi-Kiss Pure Rogue
Toradora! (best Tsundere in existence resides here)
Welcome to the N.H.K. (I think any of us shut-ins or previous shut-ins can enjoy this to no end)
Suzuka (classic)
Mirai Nikki (get over the male and female lead being annoying, it's awesome) Yandere - Yandere - Yandere
Kokoro Connect (more "psychological", it takes some episodes to realize that, but has a lot of romance done in a none typical fashion; it'll be a classic)
Chuunibyou demo Koi ga Shitai! (just... amazing, and most everyone is crazy, but in a delusional fashion not Yandere style)
I could go on for a while, so if you like my suggestions just let me know and I'll give you more later. If you don't like most of those, then I'm afraid I'll be of no use.
As for taking a stab in other areas, I'll list some of my absolute favorites in the "smart" and "psychological" categories.
Bakemonogatari
Nisemonogatari
Those two are very abstract, which I love, but the writing is... unique and amazing. There is no other writer on the planet like Nisio Isin, he's a world wonder.
Madoka Magica (don't quit after 2 episodes thinking it's your typical cutesy Mahou Shojo - DO NOT DO IT)
Steins;Gate (the only time travel anime, or hell, anything, done right)
Un-Go (if you like detective style anime - I have a lot of stuff like this to recommend)
I'll touch on Bajaratt's picks too. Jormungand is incredibly badass (if you dig it, check out Black Lagoon S1 and S2). Guilty Crown -was- fantastic, and then it ended in a rush (more like the last half of the story), it's like the writer just got tired mid-way through. That said, the journey was fun. Sword Art Online is great if, and only if, you haven't read it. I had already read it, so for me, it was to hasty and not as fleshed out as it should have been. I enjoyed watching it, but when it was over, I was really, really glad for it to be done. The second season arc was, well, like Guilty Crown, it was too fast and poorly done, though if you haven't read it, you probably wont notice this. I didn't watch Boobie Pirates, but I wont deny it seems decent enough, it's just not my cup of tea. It's fairly popular at the very least, in America (somehow).
And then I have some rather long winded posts above this about other things, some of these included. Anyway, this should get you at least a few worth watching, let me know when you run dry or want more information.